468f Solution of the Boltzmann Equation by the Fcmom

Matteo Strumendo and Hamid Arastoopour. Department of Chemical and Biological Engineering, Illinois Institute of Technology, Chicago, IL 60616

The fluid dynamics of the particulate phase in gas-solid flows (in fast and relatively dilute conditions) is described by the Boltzmann equation. Several methods are available to solve the Boltzmann equation, i.e. generalizations of the Chapman-Enskog expansion, method of moments, Monte Carlo simulations, discretization of the Boltzmann equation in the velocity space, Lagrangian methods; in this work, the focus is on the solution of the Boltzmann equation by the method of moments.

The first application of the method of moments to the Boltzmann equation was developed by Grad [1], who solved the Boltzmann equation for simple (elastic) gases using a third order approximation of the particle velocity distribution. Strumendo and Canu [2] generalized the Grad approach and were able to compute the anisotropy of the granular flows, however their technique is not successful when extended to higher order moments.

The Boltzmann equation can be interpreted as a tri-variate population balance equation, in which the internal variables are the three components of the particle velocities. In this perspective, concepts and techniques developed in the solution of population balance equations can be used for the solution of the Boltzmann equation, and vice versa.

Recently, several variations of the method of moments (QMOM, DQMOM, FCMOM) were developed and were capable to provide numerically efficient and accurate solutions of population balance equations. It is interesting to investigate whether and to which extent such techniques can be applied for solving the Boltzmann equation.

Fox [3] explored the possibility of applying quadrature-based closures in the solution of the kinetic equation for dilute gas-particle flows, thus enlarging the spectrum of applications of some of the core ideas of the QMOM/DQMOM techniques.

In this work, the FCMOM technique is extended for solving the kinetic equation representing the fluid dynamics of the particulate phase. The FCMOM (Finite size domain Complete set of trial functions Method Of Moments) was developed by Strumendo and Arastoopour ([4], [5]) to solve mono-variate and bi-variate population balance equations. The fundamental idea is to construct a method of moments on a finite domain of the internal variables (typically the particle size in mono-variate population balance equations, or the particle velocities in the kinetic equation). An advantage of the FCMOM is that it provides both the moments and the reconstructed particle distribution evolution. Further, the domain of the internal variables is always well defined (a property which is relevant in multi-variate applications).

The proposed method is illustrated through applications to the Riemann problem and to the relaxation of Maxwellian molecules.

[1] Grad, H., “On the Kinetic Theory of Rarified Gases”, Communications on Pure and Applied Mathematics, 2, 331-407, (1949).

[2] Strumendo, M., Canu P., “Method of Moments for the Dilute Granular flow of Inelastic Spheres”, Physical Review E 66, 041304/1-041304/20, (2002).

[3] Fox, R.O., “A quadrature-based third-order moment method for dilute gas-particle flows”, Journal of Computational Physics, Volume 227, Issue 12, 6313-6350, (2008).

[4] Strumendo, M., Arastoopour, H., “Solution of PBE by MOM in Finite Size Domains”, Chemical Engineering Science”, doi: 10.1016/j.ces.2008.02.010, (2008).

[5] Strumendo, M., Arastoopour, H., “Solution of Bivariate Population Balance Equations Using the FCMOM”, submitted to Industrial and Engineering Chemistry.